Direkt zum Inhalt

Ito, Suguru ; Schüler, M. ; Meierhofer, Manuel ; Schlauderer, Stefan ; Freudenstein, Josef ; Reimann, J. ; Afanasiev, Dmitry ; Kokh, K. A. ; Tereshchenko, O. E. ; Güdde, Jens ; Sentef, M. A. ; Höfer, U. ; Huber, Rupert

Build-up and dephasing of Floquet-Bloch bands on subcycle timescales

Ito, Suguru, Schüler, M., Meierhofer, Manuel , Schlauderer, Stefan, Freudenstein, Josef , Reimann, J., Afanasiev, Dmitry , Kokh, K. A., Tereshchenko, O. E. , Güdde, Jens, Sentef, M. A., Höfer, U. und Huber, Rupert (2023) Build-up and dephasing of Floquet-Bloch bands on subcycle timescales. Nature 616 (7958), S. 696-701.

Veröffentlichungsdatum dieses Volltextes: 11 Mai 2023 13:05
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.54187


Zusammenfassung

Strong light fields have created opportunities to tailor novel functionalities of solids(1-5). Floquet-Bloch states can form under periodic driving of electrons and enable exotic quantum phases(6-15). On subcycle timescales, lightwaves can simultaneously drive intraband currents(16-29) and interband transitions(18,19,30,31), which enable high-harmonic generation(16,18,19,21,22,25,28-30) and pave ...

Strong light fields have created opportunities to tailor novel functionalities of solids(1-5). Floquet-Bloch states can form under periodic driving of electrons and enable exotic quantum phases(6-15). On subcycle timescales, lightwaves can simultaneously drive intraband currents(16-29) and interband transitions(18,19,30,31), which enable high-harmonic generation(16,18,19,21,22,25,28-30) and pave the way towards ultrafast electronics. Yet, the interplay of intraband and interband excitations and their relation to Floquet physics have been key open questions as dynamical aspects of Floquet states have remained elusive. Here we provide this link by visualizing the ultrafast build-up of Floquet-Bloch bands with time-resolved and angle-resolved photoemission spectroscopy. We drive surface states on a topological insulator(32,33) with mid-infrared fields-strong enough for high-harmonic generation-and directly monitor the transient band structure with subcycle time resolution. Starting with strong intraband currents, we observe how Floquet sidebands emerge within a single optical cycle; intraband acceleration simultaneously proceeds in multiple sidebands until high-energy electrons scatter into bulk states and dissipation destroys the Floquet bands. Quantum non-equilibrium calculations explain the simultaneous occurrence of Floquet states with intraband and interband dynamics. Our joint experiment and theory study provides a direct time-domain view of Floquet physics and explores the fundamental frontiers of ultrafast band-structure engineering.



Beteiligte Einrichtungen


Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftNature
Verlag:NATURE PORTFOLIO
Ort der Veröffentlichung:BERLIN
Band:616
Nummer des Zeitschriftenheftes oder des Kapitels:7958
Seitenbereich:S. 696-701
Datum12 April 2023
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Identifikationsnummer
WertTyp
10.1038/s41586-023-05850-xDOI
Stichwörter / KeywordsHIGH-HARMONIC GENERATION; TOPOLOGICAL INSULATOR; STATES
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenZum Teil
Dokumenten-ID54187

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