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Twist- and gate-tunable proximity spin-orbit coupling, spin relaxation anisotropy, and charge-to-spin conversion in heterostructures of graphene and transition-metal dichalcogenides

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Zollner, Klaus ; João, Simão M. ; Nikolić, Branislav K. ; Fabian, Jaroslav
[img]License: Creative Commons Attribution 4.0
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Date of publication of this fulltext: 07 Dec 2023 06:05


We present a DFT-based investigation of the twist-angle dependent proximity spin-orbit coupling (SOC) in graphene/TMDC structures. We find that for Mo-based TMDCs the proximity valley-Zeeman SOC exhibits a maximum at around 15--20°, and vanishes at 30°, while for W-based TMDCs we find an almost linear decrease of proximity valley-Zeeman SOC when twisting from 0° to 30°. The induced Rashba SOC is ...


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