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Synthesis and pharmacological properties of new tetracyclic forskolin analogues

Egger, Michael ; Maity, Prantik ; Hübner, Melanie ; Seifert, Roland ; König, Burkhard


New tetracyclic analogues of forskolin have been prepared by derivatization of the natural product. Treatment of a forskolin-derived cyclic thionocarbonate with 1,3-dimethyl-2-phenyl-1,3,2-diazaphospholidine resulted in the formation of a seven-membered cyclic carbonate derivative by an unprecedented rearrangement of an intermediate dialkoxycarbene or 1,3-dipole, whereas radical deoxygenation was ...


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