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Strong coupling theory for tunneling and vibrational relaxation in driven bistable systems
Thorwart, M., Grifoni, Milena und Hänggi, P. (2001) Strong coupling theory for tunneling and vibrational relaxation in driven bistable systems. Annals of physics 293, S. 15-66.Veröffentlichungsdatum dieses Volltextes: 18 Sep 2009 09:38
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DOI zum Zitieren dieses Dokuments: 10.5283/epub.9475
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Zusammenfassung
A study of the dynamics of a tunneling particle in a driven bistable potential which is moderately-to-strongly coupled to a bath is presented. Upon restricting the system dynamics to the Hilbert space spanned by the M lowest energy eigenstates of the bare static potential, a set of coupled non-Markovian master equations for the diagonal elements of the reduced density matrix, within the discrete ...
A study of the dynamics of a tunneling particle in a driven bistable potential which is moderately-to-strongly coupled to a bath is presented. Upon restricting the system dynamics to the Hilbert space spanned by the M lowest energy eigenstates of the bare static potential, a set of coupled non-Markovian master equations for the diagonal elements of the reduced density matrix, within the discrete variale representation, is derived. The resulting dynamics
is in good agreement with predictions of ab-initio real-time path integral simulations. Numerous results, analytical as well as numerical, for the quantum
relaxation rate and for the asymptotic populations are presented. Our method is particularly convenient to investigate the case of shallow, time-dependent potential barriers and moderate-to-strong damping, where both a semi-classical and a Redfield-type approach are inappropriate.
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| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Annals of physics | ||||
| Verlag: | New York: Elsevier | ||||
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| Band: | 293 | ||||
| Seitenbereich: | S. 15-66 | ||||
| Datum | 2001 | ||||
| Institutionen | Physik > Institut für Theoretische Physik > Lehrstuhl Professor Grifoni > Arbeitsgruppe Milena Grifoni | ||||
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| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Nie, das Dokument wird nicht wissenschaftlich begutachtet werden | ||||
| An der Universität Regensburg entstanden | Unbekannt / Keine Angabe | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-94758 | ||||
| Dokumenten-ID | 9475 |

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