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One-megadalton metalloenzyme complex inGeobacter metallireducensinvolved in benzene ring reduction beyond the biological redox window

Huwiler, Simona G. ; Löffler, Claudia ; Anselmann, Sebastian E. L. ; Stärk, Hans-Joachim ; von Bergen, Martin ; Flechsler, Jennifer ; Rachel, Reinhard ; Boll, Matthias


Reversible biological electron transfer usually occurs between redox couples at standard redox potentials ranging from +0.8 to -0.5 V. Dearomatizing benzoyl-CoA reductases (BCRs), key enzymes of the globally relevant microbial degradation of aromatic compounds at anoxic sites, catalyze a biological Birch reduction beyond the negative limit of this redox window. The structurally characterized ...


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